Synthesis of Heterocycles via Multicomponent Reactions II by Géraldine Masson, Luc Neuville (auth.), Romano V. A. Orru,

By Géraldine Masson, Luc Neuville (auth.), Romano V. A. Orru, Eelco Ruijter (eds.)

Géraldine Masson, Luc Neuville ∙ Carine Bughin ∙ Aude Fayol ∙ Jieping Zhu Multicomponent Syntheses of Macrocycles Thomas J.J. Müller Palladium-Copper Catalyzed Alkyne Activation as an access to Multicomponent Syntheses of Heterocycles Rachel Scheffelaar ∙ Eelco Ruijter ∙ Romano V.A. Orru Multicomponent response layout suggestions: in the direction of Scaffold and Stereochemical range Nicola Kielland ∙ Rodolfo Lavilla contemporary advancements in Reissert-Type Multicomponent Reactions Jitender B. Bariwal ∙ Jalpa C. Trivedi ∙ Erik V. Van der Eycken Microwave Irradiation and Multicomponent Reactions Irini Akritopoulou-Zanze ∙ Stevan W. Djuric purposes of MCR-Derived Heterocycles in Drug Discovery

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1 Domino Synthesis of 2-Substituted Quinolines . . . . . . . . . . . . . . . . . . . 2 Domino Synthesis of Spiro-Benzofuranones and Spiro-Benzoindolones . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 76 9 Conclusion and Outlook . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 79 References . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .

72 8 Domino Syntheses of Heterocycles by CouplingIsomerization Sequences . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 Domino Synthesis of 2-Substituted Quinolines . . . . . . . . . . . . . . . . . . . 2 Domino Synthesis of Spiro-Benzofuranones and Spiro-Benzoindolones . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 76 9 Conclusion and Outlook .

T. J. Mu¨ller 28 1 Introduction Heterocycles are ubiquitous in all aspects of modern chemistry, such as medicinal chemistry, bioorganic and bioinorganic chemistry, and materials sciences. Their facile preparation has remained among of the most challenging goals for synthetic chemistry. However, addressing issues like simplicity, safety, brevity, selectivity, yield, environmental demands, availability of starting materials, and diversity all at the same time in the sense of an ideal synthesis [1] is an endeavor almost like squaring the circle (Fig.

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